Home
Scholarly Works
A non-reactive natural product precursor of the...
Journal article

A non-reactive natural product precursor of the duocarmycin family has potent and selective antimalarial activity

Abstract

We identify a selective nanomolar inhibitor of blood-stage malarial proliferation from a screen of microbial natural product extracts. The responsible compound, PDE-I2, is a precursor of the anticancer duocarmycin family that preserves the class's sequence-specific DNA binding but lacks its signature DNA alkylating cyclopropyl warhead. While less active than duocarmycin, PDE-I2 retains comparable antimalarial potency to chloroquine. Importantly, PDE-I2 is >1,000-fold less toxic to human cell lines than duocarmycin, with mitigated impacts on eukaryotic chromosome stability. PDE-I2 treatment induces severe defects in parasite nuclear segregation leading to impaired daughter cell formation during schizogony. Time-of-addition studies implicate parasite DNA metabolism as the target of PDE-I2, with defects observed in DNA replication and chromosome integrity. We find the effect of duocarmycin and PDE-I2 on parasites is phenotypically indistinguishable, indicating that the DNA binding specificity of duocarmycins is sufficient and the genotoxic cyclopropyl warhead is dispensable for the parasite-specific selectivity of this compound class.

Authors

Alder A; Struck NS; Xu M; Johnson JW; Wang W; Pallant D; Cook MA; Rambow J; Lemcke S; Gilberger TW

Journal

Cell Chemical Biology, Vol. 29, No. 5, pp. 840–853.e6

Publisher

Elsevier

Publication Date

May 19, 2022

DOI

10.1016/j.chembiol.2021.10.005

ISSN

2451-9456

Contact the Experts team