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Molecular Orbital Theory for Infinite Systems:...
Journal article

Molecular Orbital Theory for Infinite Systems: Hydrogen-Bonded Molecular Crystals

Abstract

In a previous paper a self consistent field (SCF) perturbation theory of the interaction between two molecules of a dimer was given. We now extend this theory to molecular crystals, with special reference to hydrogen bonded systems. The theory derived is used to calculate the geometry and energy for an infinite chain of HF molecules. The theory is checked by comparing the results obtained from some direct CNDO calculations. Calculations are …

Authors

Bacon J; Santry DP

Journal

The Journal of Chemical Physics, Vol. 56, No. 5, pp. 2011–2016

Publisher

AIP Publishing

Publication Date

March 1, 1972

DOI

10.1063/1.1677491

ISSN

0021-9606