MS-Derived Isotopic Fine Structure Reveals Forazoline A as a Thioketone-Containing Marine-Derived Natural Product Journal Articles uri icon

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abstract

  • Forazoline A is a structurally complex PKS-NRPS hybrid produced by marine-derived Actinomadura sp. During the course of studies highlighting the application of IFS analysis as a powerful tool for natural products analysis, we were alerted to an earlier misinterpretation with respect to forazoline A structure elucidation. In particular, IFS reveals that forazoline A contains a thioketone moiety rarely seen in secondary metabolites and, thus, constitutes an even more intriguing structure than originally thought.

authors

  • Zhang, Fan
  • Wyche, Thomas P
  • Zhu, Yanlong
  • Braun, Doug R
  • Yan, Jia-Xuan
  • Chanana, Shaurya
  • Ge, Ying
  • Guzei, Ilia A
  • Chevrette, Marc G
  • Currie, Cameron
  • Thomas, Michael G
  • Rajski, Scott R
  • Bugni, Tim S

publication date

  • February 21, 2020