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Journal article

Challenges in Synthesis and Analysis of Asymmetrically Grafted Cellulose Nanocrystals via Atom Transfer Radical Polymerization

Abstract

When cellulose nanocrystals (CNCs) are isolated from cellulose microfibrils, the parallel arrangement of the cellulose chains in the crystalline domains is retained so that all reducing end-groups (REGs) point to one crystallite end. This permits the selective chemical modification of one end of the CNCs. In this study, two reaction pathways are compared to selectively attach atom-transfer radical polymerization (ATRP) initiators to the REGs of …

Authors

Delepierre G; Heise K; Malinen K; Koso T; Pitkänen L; Cranston ED; Kilpeläinen I; Kostiainen MA; Kontturi E; Weder C

Journal

Biomacromolecules, Vol. 22, No. 6, pp. 2702–2717

Publisher

American Chemical Society (ACS)

Publication Date

June 14, 2021

DOI

10.1021/acs.biomac.1c00392

ISSN

1525-7797