Cu63(2) nuclear quadrupole and nuclear magnetic resonance studies of YBa2Cu4O8 in the normal and superconducting states

We report nuclear quadrupole resonance (NQR) and nuclear magnetic resonance (NMR) measurements of the spin lattice and Gaussian spin-spin relaxation times, T1 and T2G, respectively, in an unaligned (NQR) and aligned (NMR) powder of YBa2Cu4O8. Experimental details, critical for accurate NQR measurements in this system, are discussed. The normal-state data are analyzed using several models. Evidence for the existence of a spin gap is presented. …