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Dimethylmalonyltrialkylphosphoranes: New General...
Journal article

Dimethylmalonyltrialkylphosphoranes: New General Reagents for Esterification Reactions Allowing Controlled Inversion or Retention of Configuration on Chiral Alcohols

Abstract

A new class of trialkylphosphorane has been prepared through reaction of a trialkylphosphine with 2-chlorodimethylmalonate in the presence of triethylamine. These new reagents promote the condensation reaction of carboxylic acids with alcohols to provide esters along with trialkylphosphine oxide and dimethylmalonate. The condensation reaction of chiral secondary alcohols can be controlled to give either high levels of inversion or retention …

Authors

McNulty J; Capretta A; Laritchev V; Dyck J; Robertson AJ

Journal

The Journal of Organic Chemistry, Vol. 68, No. 4, pp. 1597–1600

Publisher

American Chemical Society (ACS)

Publication Date

February 1, 2003

DOI

10.1021/jo026639y

ISSN

0022-3263