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Thermodynamic and NMR analysis of inhibitor...
Journal article

Thermodynamic and NMR analysis of inhibitor binding to dihydrofolate reductase

Abstract

Isothermal titration calorimetry (ITC) was used to determine the thermodynamic driving force for inhibitor binding to the enzyme dihydrofolate reductase (DHFR) from Escherichia coli. 1,4-Bis-{[N-(1-imino-1-guanidino-methyl)]sulfanylmethyl}-3,6-dimethyl-benzene (1) binds DHFR:NADPH with a K(d) of 13±5 nM while the related inhibitor 1-{[N-(1-imino-guanidino-methyl)]sulfanylmethyl}-3-trifluoromethyl-benzene (2) binds DHFR:NADPH with a K(d) of …

Authors

Batruch I; Javasky E; Brown ED; Organ MG; Johnson PE

Journal

Bioorganic & Medicinal Chemistry, Vol. 18, No. 24, pp. 8485–8492

Publisher

Elsevier

Publication Date

December 2010

DOI

10.1016/j.bmc.2010.10.048

ISSN

0968-0896