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Polyferrocenylsilane Microspheres: Synthesis,...
Journal article

Polyferrocenylsilane Microspheres: Synthesis, Mechanism of Formation, Size and Charge Tunability, Electrostatic Self-Assembly, and Pyrolysis to Spherical Magnetic Ceramic Particles

Abstract

Pt(0)-catalyzed ring-opening precipitation copolymerization of [1]silaferrocenophanes fcSiMe(2) (3) and the spirocyclic cross-linker fcSi(CH(2))(3) (4) (fc = Fe(eta(5)-C(5)H(4))(2)) was used to prepare polyferrocenylsilane microspheres (PFSMSs) under mild conditions. By varying the reaction conditions, a wide variety of other morphologies was obtained. The effects of temperature, monomer ratio, solvent composition, catalyst concentration, and …

Authors

Kulbaba K; Cheng A; Bartole A; Greenberg S; Resendes R; Coombs N; Safa-Sefat A; Greedan JE; Stöver HDH; Ozin GA

Journal

Journal of the American Chemical Society, Vol. 124, No. 42, pp. 12522–12534

Publisher

American Chemical Society (ACS)

Publication Date

October 1, 2002

DOI

10.1021/ja0202053

ISSN

0002-7863