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Spin frustration and magnetic ordering in...
Journal article

Spin frustration and magnetic ordering in triangular lattice antiferromagnet Ca3CoNb2O9**Project supported by the National Natural Science Foundation of China (Grant Nos. 11374364 and 11222433), the National Basic Research Program of China (Grant No. 2011CBA00112). Research at McMaster University supported by the Natural Sciences and Engineering Research Council. Work at North China Electric Power University supported by the Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry.

Abstract

We synthesized a quasi-two-dimensional distorted triangular lattice antiferromagnet Ca3CoNb2O9, in which the effective spin of Co2+ is 1/2 at low temperatures, whose magnetic properties were studied by dc susceptibility and magnetization techniques. The x-ray diffraction confirms the quality of our powder samples. The large Weiss constant θCW∼ −55 K and the low Neel temperature TN∼ 1.45 K give a frustration factor f = | θCW/TN | ≈ 38, suggesting that Ca3CoNb2O9 resides in strong frustration regime. Slightly below TN, deviation between the susceptibility data under zero-field cooling (ZFC) and field cooling (FC) is observed. A new magnetic state with 1/3 of the saturate magnetization Ms is suggested in the magnetization curve at 0.46 K. Our study indicates that Ca3CoNb2O9 is an interesting material to investigate magnetism in triangular lattice antiferromagnets with weak anisotropy.

Authors

Dai J; Zhou P; Wang P-S; Pang F; Munsie TJ; Luke GM; Zhang J-S; Yu W-Q

Journal

Chinese Physics B, Vol. 24, No. 12,

Publisher

IOP Publishing

Publication Date

December 24, 2015

DOI

10.1088/1674-1056/24/12/127508

ISSN

1674-1056

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