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Rapid Assembly of Complex 3D Siloxane...
Journal article

Rapid Assembly of Complex 3D Siloxane Architectures

Abstract

Few routes to well-defined 3D silicone structures exist because of their susceptibility to depolymerization/metathesis in the presence of acids or bases. The Lewis acid B(C6F5)3 can be employed to condense hydrosilanes with alkoxysilanes, producing siloxanes and alkanes (R3SiH+R'OSiR' '3 --> R3SiOSiR' '3 + R'H). We demonstrate that balancing the steric demands at both the hydrosilane and alkoxysilanes, and the careful control of reaction …

Authors

Thompson DB; Brook MA

Journal

Journal of the American Chemical Society, Vol. 130, No. 1, pp. 32–33

Publisher

American Chemical Society (ACS)

Publication Date

January 1, 2008

DOI

10.1021/ja0778491

ISSN

0002-7863