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Understanding the Effect of Ni-Substitution on the...
Journal article

Understanding the Effect of Ni-Substitution on the Oxygen Evolution Reaction of (100) IrO2 Surfaces

Abstract

The electrolysis process of water is impeded by the slow kinetics of the oxygen evolution reaction (OER). While iridium oxide (IrO2) is considered one of the most efficient metal catalysts for the OER, the adsorption of the OER intermediates at the IrO2 surface is not optimal, the *OH intermediate being too strongly adsorbed. The substitution of iridium by another metal cation is then a common strategy to improve the catalytic activity. A …

Authors

Buvat G; Eslamibidgoli MJ; Zhang T; Prabhudev S; Youssef AH; Ruediger A; Garbarino S; Botton GA; Zhang P; Eikerling M

Journal

ACS Catalysis, Vol. 12, No. 17, pp. 10961–10972

Publisher

American Chemical Society (ACS)

Publication Date

September 2, 2022

DOI

10.1021/acscatal.2c02591

ISSN

2155-5435