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Determination of the Bonding and Valence...
Journal article

Determination of the Bonding and Valence Distribution in Inorganic Solids by the Maximum Entropy Method

Abstract

The distribution of valence among the bonds in the bond graph of an inorganic compound is used to calculate an `entropy'. We show that the distribution of valence that maximizes this entropy (ME) is similar, but not identical, to that obtained using the equal-valence rule (EVR) proposed by Brown [Acta Cryst. (1977), B33, 1305–1310]. Since the ME solutions are maximally non-committal with regard to missing information, they give better …

Authors

Rao GH; Brown ID

Journal

Acta Crystallographica Section B: Structural Science, Crystal Engineering and Materials, Vol. 54, No. 3, pp. 221–230

Publisher

International Union of Crystallography (IUCr)

Publication Date

June 1, 1998

DOI

10.1107/s0108768197013426

ISSN

2052-5192