Journal article
Selective reduction of CO to acetaldehyde with CuAg electrocatalysts
Abstract
Electrochemical CO reduction can serve as a sequential step in the transformation of CO2 into multicarbon fuels and chemicals. In this study, we provide insights on how to steer selectivity for CO reduction almost exclusively toward a single multicarbon oxygenate by carefully controlling the catalyst composition and its surrounding reaction conditions. Under alkaline reaction conditions, we demonstrate that planar CuAg electrodes can reduce CO …
Authors
Wang L; Higgins DC; Ji Y; Morales-Guio CG; Chan K; Hahn C; Jaramillo TF
Journal
Proceedings of the National Academy of Sciences of the United States of America, Vol. 117, No. 23, pp. 12572–12575
Publisher
Proceedings of the National Academy of Sciences
Publication Date
June 9, 2020
DOI
10.1073/pnas.1821683117
ISSN
0027-8424