We study the pump-probe response of three insulating cuprates and develop a
model for its recombination kinetics. The dependence on time, fluence, and both
pump and probe photon energies imply many-body recombination on femtosecond
timescales, characterized by anomalously large trapping and Auger coefficients.
The fluence dependence follows a universal form that includes a characteristic
volume scale, which we associate with the holon-doublon excitation efficiency.
This volume varies strongly with pump photon energy and peaks near twice the
charge-transfer energy, suggesting that the variation is caused by carrier
multiplication through impact ionization.
Authors
Sahota DG; Liang R; Dion M; Fournier P; DÄ…bkowska HA; Luke GM; Dodge JS