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Spin-Singlet Ground State of Two-Dimensional...
Journal article

Spin-Singlet Ground State of Two-Dimensional Quantum Spin Antiferromagnet (CuCl)Ca2Nb3O10

Abstract

We report structural and magnetic properties of the triple-layered perovskite (CuCl)Ca2Nb3O10 with a spin-1/2 CuCl layer, investigated by transmission electron microscopy, magnetic susceptibility, high-field magnetization, specific heat, µSR, and inelastic neutron scattering measurements. The results show that (CuCl)Ca2Nb3O10 has a spin-singlet ground state with a gap of Δ/kB = 11 K. The observation of a 2 × 2 superstructure suggests a coherent …

Authors

Tsujimoto Y; Kitada A; Nishi M; Narumi Y; Kindo K; Goko T; Uemura YJ; Aczel AA; Williams TJ; Luke GM

Journal

Journal of the Physical Society of Japan, Vol. 83, No. 7,

Publisher

Physical Society of Japan

Publication Date

July 15, 2014

DOI

10.7566/jpsj.83.074712

ISSN

0031-9015