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Journal article

Charge Density Wave Order and Fluctuations above TCDW and below Superconducting Tc in the Kagome Metal CsV3Sb5

Abstract

The phase diagram of the kagome metal family AV_{3}Sb_{5} (A=K, Rb, Cs) features both superconductivity and charge density wave (CDW) instabilities, which have generated tremendous recent attention. Nonetheless, significant questions remain. In particular, the temperature evolution and demise of the CDW state has not been extensively studied, and little is known about the coexistence of the CDW with superconductivity at low temperatures. We report an x-ray scattering study of CsV_{3}Sb_{5} over a broad range of temperatures from 300 to ∼2  K, below the onset of its superconductivity at T_{c}∼2.9  K. Order parameter measurements of the 2×2×2 CDW structure show an unusual and extended linear temperature dependence onsetting at T^{*}∼160  K, much higher than the susceptibility anomaly associated with CDW order at T_{CDW}=94  K. This implies strong CDW fluctuations exist to ∼1.7×T_{CDW}. The CDW order parameter is observed to be constant from T=16 to 2 K, implying that the CDW and superconducting order coexist below T_{c}, and, at ambient pressure, any possible competition between the two order parameters is manifested at temperatures well below T_{c}, if at all. Anomalies in the temperature dependence in the lattice parameters coincide with T_{CDW} for c(T) and with T^{*} for a(T).

Authors

Chen Q; Chen D; Schnelle W; Felser C; Gaulin BD

Journal

Physical Review Letters, Vol. 129, No. 5,

Publisher

American Physical Society (APS)

Publication Date

July 29, 2022

DOI

10.1103/physrevlett.129.056401

ISSN

0031-9007

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