Binder migration during drying of lithium-ion battery electrodes: Modelling and comparison to experiment

The drying process is a crucial step in electrode manufacture that may lead to spatial inhomogeneities in the distribution of the electrode components resulting in impaired cell performance. Binder migration during the drying process, and the ensuing poor binder coverage in certain regions of the electrode, can lead to capacity fade and mechanical failure (e.g. electrode delamination from the current collector). A mathematical model of …